Fast Flowing Heat in Graphene Heterostructures

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Nanoscale heat flow plays a crucial role in many modern electronic and optoelectronic applications, such as thermal management, photodetection, thermoelectrics and data communication. Two-dimensional layered materials are beginning to confirm their groundbreaking role in many of these applications. Perhaps even more promising are so-called van der Waals heterostructures, consisting of different layered two-dimensional materials stacked one on top of the other. These stacks can consist of materials with dramatically different physical properties, while the interfaces between them are ultraclean and atomically sharp.

Scientists from the European Graphene Flagship, led by ICFO researchers, have recently succeeded in observing and following, in real-time, the way in which heat transport occurs in van der Waals stacks, which consist of graphene encapsulated by the dielectric two-dimensional material hexagonal BN (hBN).

In a study, recently published in Nature Nanotechnology entitled “Out-of-plane heat transfer in van der Waals stacks through electron–hyperbolic phonon coupling” , ICFO researchers Klaas-Jan Tielrooij, Niels C. H. Hesp, Mark B. Lundeberg, Mathieu Massicotte, Peter Schmidt, and Diana Davydovskaya, led by ICREA Prof at ICFO Frank Koppens, in collaboration with researchers from The Netherlands, Italy, Germany, and United Kingdom, have identified a highly surprisingly effect: rather than staying within the graphene sheet, the heat actually flows to the surrounding hBN sheets. This out-of-plane heat transfer process occurs on an ultrafast timescale of picoseconds (one millionth of a millionth of a second), and is therefore dominant over competing (in-plane) heat transfer processes.

The heat transfer process occurs through hot graphene electrons (experimentally generated by incident light) that couple to hyperbolic phonon-polaritons in the hBN sheets. These phonon-polaritons propagate within the hBN as light does in an optical fiber, but in this case for infrared wavelengths and at the nanometer scale. It turns out that these exotic hyperbolic modes are very efficient at carrying heat away.

The results of this work will definitely have far-reaching implications for many applications based on hBN-encapsulated graphene, sometimes referred to as the next generation graphene platform, owing to its superior electrical properties. In particular, it will provide direction to optoelectronic device design, where these heat flow processes can be thoroughly exploited.